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Regensburg 2000 – wissenschaftliches Programm

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TT: Tiefe Temperaturen

TT 7: Postersitzung I: Amorphe- und Tunnelsysteme (1-8), Mesoskopische Systeme (9-21), Schwere Fermionen (22-32), Kernmagnetismus (33-34), Josephson-Kontakte und SQUIDs (35-45), TT-Detektoren und Kryotechnik (46-49)

TT 7.26: Poster

Montag, 27. März 2000, 14:30–18:00, A

Specific heat capacity of the semimetal Ce3Cu3Sb4 in magnetic fields up to 14 T — •W. Schnelle1 and R.K. Kremer21Max-Planck-Institut für Chemische Physik fester Stoffe, Dresden, Germany — 2Max-Planck-Institut für Festkörperforschung, Stuttgart, Germany

Ce3Cu3Sb4 is a cubic compound exhibiting semimetallic to semiconducting behaviour and a phase transition to a state with a spontaneous magnetic moment at ≈11 K. The specific heat capacity of Ce3Cu3Sb4 was measured between 0.6 K and 100 K in magnetic fields up to 140 kOe. The lattice contribution was estimated using the isostructural La3Cu3Sb4. The magnetic ordering transition of Ce3Cu3Sb4 at 10.85(2) K shows up as a tiny step-like anomaly in the magnetic specific heat, while the low-temperature behaviour is dominated by a broad hump centred at 4.8(1) K. With small magnetic fields (<10 kOe) the transition shifts to higher temperatures and disappears. The hump at low T broadens and shifts to higher temperatures with the increase of the magnetic field to 140 kOe. Our results are discussed in the context of a recent determination of the magnetic structure of Ce3Cu3Sb4 which indicates a magnetic ordering with the full saturated theoretical Ce3+ moment.

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