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DPG

Berlin 2001 – scientific programme

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A: Atomphysik

A 12: Posters Thursday (Ion/Atom/Molecule/Surface Scattering)

A 12.34: Poster

Thursday, April 5, 2001, 12:30–15:00, AT3

Anisotropy of the KCO normal interaction potential at 1   eV and activation energy of the (0→ 1) vibrational excitation of CO scattered by K — •Karsten Rott and Dieter Beck — Universität Bielefeld, Universitätsstasse 25, D-33615 Bielefeld

We analysed the anisotropy of the KCO interaction potential at V ≈ 1 eV by performing scattering experiments with crossed molecular beams. The energetically and angularly resolved differential cross section was measured and the rotational inelastic scattering was simulated using the classical hard shell model. A shell shaped like an egg with its thin, more curved end in oxygen direction gives good results in comparison with experiment.

Vibrational excitation is found to set in as the (0 → 1) transition at the collision energy E = 1.0   eV . It is apparently caused by the avoided crossing of the X2 A′ and A2 A′ potentials of KCO .

Comparing similar systems KCO and KN2 we also find very different, hitherto unexplained yields of vibrational excitation of the molecules and electronical excitation of K .

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