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Regensburg 2004 – wissenschaftliches Programm

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MA: Magnetismus

MA 13: Poster:Schichten(1-23),Spinabh.Trsp(24-41),Exch.Bias(42-56),Spindyn.(57-67),Mikromag.(68-76),Partikel(77-90),Spinelektr.(91-97),Elektr.Theo.(98-99),Mikromag+PhasÜ+Aniso.(100-105),Magn.Mat.(106-118),Messmethod.(119-121),Obflm.+Abbverf.(122-123)

MA 13.94: Poster

Dienstag, 9. März 2004, 15:00–19:00, Bereich A

Cobalt doping of a low-energy interface in anatase — •Michael Schreiber1, Rebecca Janisch1,2, Sibylle Gemming1, and Nicola Spaldin21Institut für Physik, Technische Universität, 09107 Chemnitz, Germany — 2Materials Research Laboratory, University of California, Santa Barbara CA 93106, USA

About two years ago Co-doped TiO2 anatase has been discovered to exhibit ferromagnetism at and above room temperature, i.e. to be a magnetically robust diluted magnetic semiconductor (DMS). Since then it has attracted considerable interest, but there is still controversy over the origin of the magnetism as well as the influencing factors.
In this work a low-energy Σ5(113)[-110] grain boundary in anatase is studied by density-functional band-structure calculations employing norm-conserving pseudopotentials and plane waves [1].
The interfacial structure in pure anatase exhibits close structural and electronic similarity to the pure bulk anatase crystal. Yet, the grain boundary acts as a sink for dopant atoms, such as Co. This result confirms the importance of the investigation of grain boundaries in the discussion of DMS properties. The influence of inner interfaces on the magnetic properties of Co-doped TiO2 is subject to ongoing investigations, the results of which will be shown on the poster.

[1] The ABINIT code is a common project of the Université Catholique de Louvain, Corning Inc., and other contributors (URI http://www.abinit.org).

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