Berlin 2005 – scientific programme
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TT: Tiefe Temperaturen
TT 16: Posters Correlated Electrons, Measuring Devices, Cryotechnique
TT 16.68: Poster
Saturday, March 5, 2005, 11:00–16:30, Poster TU C
Itinerant electron metamagnetism and weak ferromagnetism in LaCo9Si4 and YCo9Si4 — •H. Michor1, S. Özcan1, M. El-Hagary1, E. Bauer1, M. Reissner1, G. Hilscher1, S. Khmelevskyi2, P. Mohn2, P. Rogl3, and H. Rosner4 — 1Institut für Festkörperphysik, T.U. Wien, A-1040 Wien, Austria — 2Center for Computational Materials Science, T.U. Wien, Austria — 3Institut für Physikalische Chemie, Universität Wien, Austria — 4Max-Planck Institute for Chemical Physics of Solids, D-01187 Dresden, Germany
LaCo9Si4 is a strongly exchange enhanced Pauli paramagnet with an instability towards weak ferromagnetism, i.e. exhibits itinerant electron metamagnetism at about 3.5 T for H||c and 6 T for H⊥ c, which is the lowest value ever found for rare earth intermetallic compounds [1]. Despite of the smaller unit cell volume isostructural and isoelectronic YCo9Si4 exhibits a weak itinerant ferromagnetic ground state (TC≃ 25 K) already in zero-field. The ground state properties of La- and YCo9Si4 are discussed on basis of magnetisation, specific heat, and resistivity measurements and via ab-initio electronic structure calculations. The band structure calculations result in a ferromagnetic groundstate for both compounds with moments substantialy larger than the experimentally observed moments. The origin of these discrepancies is briefly discussed. [1] H. Michor et al., Phys.Rev. B 69 (2004) 081404(R).