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Dresden 2009 – wissenschaftliches Programm

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O: Fachverband Oberflächenphysik

O 38: Nano-optics of metallic and semiconducting nanostructures (experiments I)

O 38.3: Vortrag

Mittwoch, 25. März 2009, 15:30–15:45, SCH A216

Antenna enhanced Pump-Probe Spectroscopy of Single Metal Nanoparticles — •David Molnar1,2 and Markus Lippitz1,21Max-Planck-Institut für Festkörperforschung, Stuttgart — 24. Physikalisches Institut, Universität Stuttgart

Tailoring a nanoparticle's properties for technological applications requires a profound understanding of its different characteristics compared to those of its bulk material. One arising question is: Down to which lengths can a material be expected to show bulk behaviour?

Acoustical eigenfrequencies of a single gold nanoparticle give insight to its mechanical properties such as density or Young's modulus. A laser induced mechanical oscillation yields a periodical change of the electron density, i.e., a periodically changing plasmon resonance. This change is optically detectable using a pump-probe technique and reveals the dynamics of the particle's oscillation.

As absorption is proportional to the third power of the particle's radius the optical detection of mechanical oscillations of a single metal particle with a diameter of 40nm or less is almost impossible. However using an adequate antenna enhancing the signal oscillations of a single particle, 10nm in size or less, become detectable.

We will show calculations of the signal enhancement by an antenna as well as first experimental results in this field.

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