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TT: Fachverband Tiefe Temperaturen
TT 25: Superconductivity: Cuprate High-Temperature Superconductors 1
TT 25.13: Vortrag
Mittwoch, 25. März 2009, 12:45–13:00, HSZ 304
Charge-Transfer Excitons In Underdoped Ca2−xNaxCuO2Cl2 — •R. Schuster1, S. Pyon2, M. Knupfer1, J. Fink1,3, M. Azuma4, M. Takano4, H. Takagi2, and B. Büchner1 — 1IFW Dresden, Institute for Solid State Research, P.O. Box 270116, D-01171 Dresden, Germany — 2Department of Advanced Materials Science, University of Tokyo, Kashiwa 277 8581, Japan — 3BESSY GmbH, Albert-Einstein-Strasse 15, 12489 Berlin, Germany — 4Inst. Chem. Res., Kyoto Univ., Uji, Kyoto-fu 611-0011, Japan
Employing electron energy-loss spectroscopy we show that small values of doping in the system Ca2−xNaxCuO2Cl2 strongly influence the formation and dynamics of charge-transfer excitons in the Cu-O plane. We find a remarkable redistribution of spectral weight between the two modes seen in the insulator yielding a single sharp feature for non-zero doping; accompanied by a strong suppression of the dispersion. Our data may provide evidence for a prominent role of the magnetic background on the dynamics of charge-transfer excitations in underdoped cuprates.