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DS: Fachverband Dünne Schichten

DS 10: Plasmonics and Nanophotonics I (Joint Session DS/O/HL)

DS 10.5: Vortrag

Dienstag, 23. März 2010, 11:30–11:45, H2

Manipulation of fluorescence resonance energy transfer in single plasmonic nanoresonators — •Valerie Faessler, Calin Hrelescu, Sergiy Mayilo, Frank Jäckel, and Jochen Feldmann — Photonics and Optoelectronics Group, Department of Physics and Center for Nano Science (CeNS), Ludwig-Maximilians-Universität München, Amalienstrasse 54, 80799 München, Germany;

We show that fluorescence resonance energy transfer (FRET) between two organic chromophores can be manipulated in plasmonic nanoresonators consisting of two spherical gold nanoparticles.The nanoresonators can be tuned by varying the inter-particle distance or the nanoparticle size. This allows us to selectively modify the decay channels of the chromophores. FRET can be supressed if the molecules are placed in the nanoresonator at a certain distance from the nanoparticle surface. Furthemore we observe spectral shaping and intensity modulation of the fluorophore emision in the nanoresonators [1]. Correlated whitelight Rayleigh scattering and fluorescence microscopy data of the hybrid system are discussed in the framework of generalized Mie theory.

[1] M. Ringler, A. Schwemer, M. Wunderlich, A. Nichtl, K. Kürzinger, T. A. Klar, J. Feldmann Phys. Rev. Lett., 100, 203002 (2008)