Regensburg 2013 – scientific programme
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MA: Fachverband Magnetismus
MA 25: Magnetic Heusler Compounds
MA 25.8: Talk
Wednesday, March 13, 2013, 11:15–11:30, H10
NMR Sheds Light on Structural Evolution upon Annealing and Off-Stoichiometry in Nominal Co2MnSi Thin Films — •Steven Rodan1, Alexey Alfonsov1, Maria-Eleni Belesi1, Filippo Ferraro2, Jürgen T. Kohlhepp2, Henk J. M. Swagten2, Bert Koopmans2, Bernd Büchner1, and Sabine Wurmehl1 — 1Leibniz Institute for Solid State and Materials Research, 01171 Dresden, Germany — 2Eindhoven University of Technology, 5600 MB Eindhoven, Netherlands
Half-metallic ferromagnets (HMFs), with fully spin-polarized conduction electrons, are prime candidates for developing spintronic devices. Many Heusler compounds, such as Co2MnSi, are predicted to be HMFs. A local probe technique such as nuclear magnetic resonance (NMR) is essential for understanding the microscopic origin of manifested physical properties, such as the magnetoresistance ratio measured in giant magnetoresistance (GMR) devices. Using NMR we have studied the evolution of local atomic structure in numerous Co2MnSi thin films prepared by different methods, subjected to various annealing temperatures, and with varying stoichiometry. For all cases, we investigated models for different types of disorder, and quantitatively deduced the off-stoichiometry. By understanding how the local structure affects the physical properties, one can hope to control and optimize the properties which are of interest for spintronics by appropriately tuning the structure.