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MA: Fachverband Magnetismus
MA 33: Magnetization Dynamics I of 3
MA 33.10: Vortrag
Donnerstag, 14. März 2013, 11:45–12:00, H22
Optically induced ultrafast spin dynamics in Au/Fe/MgO(001) structures: the role of hot carrier transport — •Alexandr Alekhin1, Damian Bürstel2, Tim O. Wehling3, Detlef Diesing2, Alexander I. Lichtenstein4, Uwe Bovensiepen5, and Alexey Melnikov1 — 1Fritz-Haber-Institut der MPG, Dep. of Phys. Chem., Berlin, Germany — 2University of Duisburg-Essen, Insitute of Phys. Chem., Essen, Germany — 3University of Bremen, Institute of Theor. Phys., Bremen, Germany — 4University of Hamburg, Institute of Theor. Phys., Hamburg, Germany — 5University of Duisburg-Essen, Dep. of Physics, Essen, Germany
Spin dynamics (SD) induced by ultrashort laser pulses is of great importance in light of recent advance in spintronics and attempts to control magnetization on femtosecond (fs) time scales. To understand the origin of ultrafast demagnetization, pump-probe experiments have been performed on epitaxial Au/Fe/MgO(001) structures. Using 14 fs laser pulses to probe the Fe side of the samples, we monitor bulk SD by the magneto-optical Kerr effect (MOKE) and SD at interfaces by the magneto-induced second harmonic generation (mSHG). To disentangle interfering mSHG contributions from different interfaces, we have analyzed the dependence of mSHG response on the thickness of Fe film. This approach gives us an access to spatially non-uniform transient magnetization. Comparison of transient mSHG response of Fe to direct optical excitation with that to excitation by hot carriers (HC) generated in Au reveals a significant contribution of spin polarized HC transport to ultrafast demagnetization.