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Dresden 2014 – wissenschaftliches Programm

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O: Fachverband Oberflächenphysik

O 37: Posters: Plasmonics, Electronic Structure and Spin-Orbit Interaction, Semiconductor and Insulator Surfaces, Nanostructures

O 37.40: Poster

Dienstag, 1. April 2014, 18:30–22:00, P2

Diffraction-limited few-cycle shaped laser pulses for plasmon microscopy — •Sebastian Goetz1, Monika Pawlowska1, Christian Dreher1, Christian Rewitz1, Enno Krauss2, Peter Geisler2, Gary Razinskas2, Bert Hecht2,3, and Tobias Brixner1,31Institut für Physikalische und Theoretische Chemie, Universität Würzburg, Am Hubland, 97074 Würzburg, Germany — 2Nano-Optics and Biophotonics Group, Experimentelle Physik 5, Universität Würzburg, Am Hubland, 97074 Würzburg, Germany — 3Röntgen Center for Complex Material Systems (RCCM), Am Hubland, 97074 Würzburg, Germany

For the investigation of ultrafast processes on the nanoscale by far-field radiation, the temporal resolution of femtosecond laser pulses has to be combined with the spatial resolution of a high-NA microscope. Both resolutions need to be conserved when the incoming light field is manipulated, which is a prerequisite for the demanding concept of coherent control. These functionalities are implemented in our group by pairing confocal microscopy with phase and amplitude pulse shaping of few-cycle NIR pulses using an LCD pulse shaper in 4f single-pass geometry. The capability of the setup is demonstrated by investigating the influence on the diffraction-limited focus of LCD imperfections and spatio-temporal coupling. We examine the laser focus on plain gold surfaces and nanostructures by spectrally and spatially resolved analysis of reflections from the sample plane.

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