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Regensburg 2016 – scientific programme

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O: Fachverband Oberflächenphysik

O 32: 2D Materials I: Structure and Electronic Properties

O 32.7: Talk

Tuesday, March 8, 2016, 12:00–12:15, H24

Spatial conductivity mapping of unprotected and capped black phosphorus using microwave microscopyPieter J. de Visser1,2, Rebekah Chua1,3, Joshua O. Island1, Matvey Finkel1,4, Allard J. Katan1, •Holger Thierschmann1, Herre S.J. van der Zant1, and Teun M. Klapwijk1,41Kavli Insitute of Nanoscience, Faculty of Applied Sciences, Delft University of Technology, The Netherlands — 2Department of Quantum Matter Physics, University of Geneva, Switzerland — 3Department of Physics, National University of Singapore, Singapore — 4Physics Department, Moscow State Pedagogical University, Russia

Within the family of 2D materials thin flakes of black Phosphorus (bP) play a special role due to their tuneable direct bandgap and high carrier mobilities. Under ambient conditions, however, degradation changes the electronic properties of bP dramatically within hours [1]. Hence, applying protection measures is essential. We compare different protecting layers by measuring the local conductivity of bP flakes over time with scanning microwave impedance microscopy (sMIM). This novel AFM-based technique [2] probes the local sheet resistance with high spatial resolution and even for buried layers. For a bare bP flake we observe drastic changes in conductivity within 24 h. Coverage with 10 nm of HfOx delays degradation. The bP flake is stable for more than a week. Boron Nitride flakes appear to be less effective as a protection. sMIM reveals that here degradation starts at the edges and evolves over days, indicating a diffusive process. [1] Island J O, et al. 2DMat 2, 011002 (2015). [2] K. Lai, et al. Rev Sci Inst 79, 063703 (2008).

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