Regensburg 2016 – wissenschaftliches Programm
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TT: Fachverband Tiefe Temperaturen
TT 43: Correlated Electrons: f-Electron & Heavy Fermion Systems
TT 43.7: Vortrag
Mittwoch, 9. März 2016, 11:00–11:15, H20
Exchange field effect in the crystal field ground state of CeMAl4Si2 — •Kai Chen1, Fabio Strigari1, Martin Sundermann1, Stefano Agrestini2, Eric D. Bauer3, John L. Sarrao3, Joe D. Thompson3, Edwige Otero4, Arata Tanaka5, and Andrea Severing1 — 1University of Cologne, Cologne, Germany — 2Max Planck Institute for Chemical Physics of Solids, Dresden, Germany — 3Los Alamos National Laboratory, Los Alamos, US — 4Synchrotron Soleil,Gif-sur-Yvette Cedex,France — 5Hiroshima University, Higashi-Hiroshima,Japan
The crystal-field ground state wave functions of the tetragonal Kondo lattice materials CeMAl4Si2(M = Rh, Ir and Pt), as well as the crystal-field splittings, are determined with low temperature linear polarized soft x-ray absorption spectroscopy. Surprisingly, at T < 20 K, which is far below the first excited crystal-field level at 200 K, a change in linear dichroism was observed that cannot be accounted for by population of crystal-field states. Adding an exchange field to the ionic full multiplet calculations below 20 K leads to a splitting to the ground state doublet and modification of Jz admixture, thus accounting for the change in low temperature linear dichroism. The direction of the required exchange field is parallel along c-axis for the antiferromagnetic Rh and Ir compounds, and perpendicular to c-axis for ferromagnetic CePtAl4Si2.