Berlin 2018 – wissenschaftliches Programm
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O: Fachverband Oberflächenphysik
O 83: Poster Focus Session: Structural Dynamics in Nanoscale Materials, Probed by Ultrafast Electron Pulses
O 83.10: Poster
Mittwoch, 14. März 2018, 18:15–20:30, Poster A
Harmonicity and anharmonicity of phonon and surface phonon-polariton in high symmetry directions in wurtzite AlN — •Hrag Karakachian1,2 and Michel Kazan1 — 1Department of Physics, American University of Beirut, P.O. Box 11-0236, Riad El-Solh, Beirut 1107-2020, Lebanon — 2Max-Planck-Institut für Festkörperforschung, Heisenbergstr. 1, 70569 Stuttgart, Germany
We report on the potential of self-nucleated AlN single crystal as a tunable near-field infrared source. The grown crystal exhibits natural AlN growth characteristics with several well-developed facets of different orientations. The characteristics of surface-phonon-polariton (SPhP) modes on the developed crystal facets have been investigated. Reflectivity spectra were recorded from five facets of different orientations. The measured spectra were analyzed by a model taking into account the dependence of harmonicity and anharmonicity of the excited zone center optical phonons on the surface orientation. Consequently, the dielectric properties that determine the condition of existence, dispersion relations, and lifetimes of the SPhP modes were accurately retrieved. The dielectric functions were determined as a function of the angle of incidence and used to compute the characteristics of the SPhP modes on each of the measured facets. We found that facets of different orientations exhibit SPhP modes of different frequencies and lifetimes, which makes the investigated self-nucleated crystal potential candidates for tunable near-field infrared sources.