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TT: Fachverband Tiefe Temperaturen
TT 47: Quantum Magnets, Molecular Magnets and Skyrmions
TT 47.8: Vortrag
Mittwoch, 3. April 2019, 17:00–17:15, H23
Quantum tunneling and large coercivity in Fe-doped Li3N — Manuel Fix1, Enrique del Barco2, and •Anton Jesche1 — 1EP VI, Center for Electronic Correlations and Magnetism, Augsburg University, 86135 Augsburg, Germany — 2Department of Physics, University of Central Florida, Orlando, Florida 32816, USA
The basic magnetic unit in Fe-doped Li3N is not a cluster or a domain but the magnetic moment of single, isolated Fe ions [1]. This novel model system shows large magnetic anisotropy and allows to study quantum tunneling of the magnetization in a rather simple, inorganic material at liquid helium temperatures.
For small concentrations of roughly 0.1 % Fe, we have found an extreme field-dependence of the magnetic tunneling [2].
Applied longitudinal fields lift the ground-state degeneracy and destroy the tunneling condition.
The relaxation time increases from τ ∼ 104 by four orders of magnitude in applied fields of only a few milliTesla, which reveals exceptionally sharp tunneling resonances.
In applied transverse magnetic fields, on the other hand, the spin-flip probability increases, which proves the resonant character of this tunneling process.
Therefore, it is possible either to freeze the orientation or to promote the flip of a spin-state by tiny applied fields.
A. Jesche et al., Nat. Commun. 5:3333 (2014)
M. Fix, J. H. Atkinson, P. C. Canfield, E. del Barco, A. Jesche, Phys. Rev. Lett. 120, 147202 (2018)