Rostock 2019 – wissenschaftliches Programm
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MO: Fachverband Molekülphysik
MO 9: Molecules in Intense Laser Fields
MO 9.3: Vortrag
Montag, 11. März 2019, 16:45–17:00, S HS 002 Biologie
Static coherent states method: one and two electron laser-induced systems with classical nuclear dynamics — •Mohammad Reza Eidi1, Mohsen Vafaee2, and Alexandra Landsman1,3 — 1Max Planck Institute for the Physics of Complex Systems, Dresden, Germany — 2Department of Chemistry, Tarbiat Modares University, Tehran, Iran — 3Max Planck Korea, Department of Physics, Postech, Pohang, Gyeongbuk 37673, Republic of Korea
In the presented work, the static coherent states method (SCS) is introduced to investigate quantum electron dynamics in a one or two-electron laser-induced system. The SCS method solves the time-dependent Schrödinger equation (TDSE) both in imaginary and real times on the base of a static grid of coherent states. Moreover, classical dynamics is considered for the nuclei by solving their Newtonian equation of motion. Implementing classical nuclear dynamics, the electronic state potential energy curves of H2+ in the absence and presence of an ultra-short intense laser field is computed. We use this method to investigate charge migration in H2+. In particular, we find that the charge migration time increases exponentially with internuclear distance. We also observe substantial charge localization for sufficiently long molecular bonds.