Regensburg 2022 – scientific programme
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MA: Fachverband Magnetismus
MA 42: Magnetic Heuslers
MA 42.5: Talk
Friday, September 9, 2022, 12:30–12:45, H48
Noncollinear magnetic order in epitaxial thin films of the MnPtGa hard magnet — •Rebeca Ibarra1,2, Edouard Lesne1, Bachir Ouladdiaf3, Ketty Beauvois3, Alexandr Sukhanov2, Rafal Wawrzyńczak1, Walter Schnelle1, Anton Devishvili3, Dmytro Inosov2, Claudia Felser1, and Anastasios Markou1 — 1Max-Planck-Institute für Chemische Physik fester Stoffe, D-01187 Dresden, Germany — 2Institut für Festkörper- und Materialphysik, Technische Universität Dresden, D-01069 Dresden, Germany — 3Institut Laue-Langevin, CS20156, 38042 Grenoble Cedex 9, France
Noncollinear magnetism has attracted great attention in the recent years and promise rich exotic properties with potential for spintronic applications. In this work, we present a detailed analysis of the structural and magnetic properties of high-quality thin films of the hexagonal MnPtGa hard magnet grown on Al2O3(0001) substrates. The films crystalize in the P63/mmc space group, with an ordering temperature of TC = 263 K into a ferromagnetic (FM) state, followed by a spin reorientation transition at Tsr ∼ 160 K. A large uniaxial magnetic anisotropy is observed in this centrosymmetric compound. We further investigate the magnetic transitions by single-crystal neutron diffraction at zero applied magnetic field. The emergence of the structurally forbidden (001) Bragg reflection for T < 160 K, unequivocally determines a transition to a spin canted state, where the Mn magnetic moments align ferromagnetically along the c-axis and antiferromagnetically in the basal plane, resulting in a spin canting angle of 20∘ respect to the c-axis.