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SAMOP 2023 – wissenschaftliches Programm

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Q: Fachverband Quantenoptik und Photonik

Q 22: Poster II

Q 22.64: Poster

Dienstag, 7. März 2023, 16:30–19:00, Empore Lichthof

Chiral Rydberg State in cold atoms for chiral sensing.Stefan Aull1, Steffen Giesen2, •Peter Zahariev1,3, Robert Berger2, and Kilian Singer11Institut für Physik, Experimentalphysik I , Universität Kassel, Heinrich-Plett-Str. 40, 34132 Kassel — 22Fb. 15 - Chemie, Hans- Meerwein-Straße 4, 35032 Marburg — 3Institute of Solid State Physics, Bulgarian Academy of Sciences, 72, Tzarigradsko Chaussee, 1784 Sofia, Bulgaria

It has been shown theoretically [1] that by combining a superposition of Hydrogenic wavefunctions in combination with appropriately adjusted phases, the resulting electronic state can show chiral properties. We are proposing a protocol for experimentally creating those states in a ultra-cold cloud of Rubidium atoms by exciting into a circular Rydberg state and subsequently generating a superposition of different states of almost maximum ℓ and m. The results are aimed to be used for chiral discrimination [2] of molecules. Optimized parameters will be determined to maximize the chiral sensitivity.

[1] A. Ordonez, O. Smirnova. Propensity rules in photoelectron circular dichroism in chiral molecules. I. Chiral hydrogen, Phys. Rev. A 99, 043416 (2019)

[2] S Y Buhmann et al, Quantum sensing protocol for motionally chiral Rydberg atoms, New J. Phys. 23, 083040 (2021)

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