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SKM 2023 – scientific programme

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O: Fachverband Oberflächenphysik

O 15: Spins on Surfaces at the Atomic Scale II

O 15.4: Talk

Monday, March 27, 2023, 15:45–16:00, REC C 213

Certifying entanglement of spins on surfaces using ESR-STM — •Yelko del Castillo1,2 and Joaquín Fernández-Rossier11International Iberian Nanotechnology Laboratory (INL), Av. Mestre José Veiga, 4715-330 Braga, Portugal — 2Centro de Física das Universidades do Minho e do Porto, Universidade do Minho, Campus de Gualtar, 4710-057 Braga, Portugal

We propose a protocol to certify the presence of entanglement in artificial on-surface atomic and molecular spin arrays using electron spin resonance carried by scanning tunnel microscopes (ESR-STM). We first generalize the theorem that relates global spin susceptibility as an entanglement witness to the case of anisotropic Zeeman interactions, relevant for surfaces. We then propose a method to measure the spin susceptibilities of surface-spin arrays combining ESR-STM with atomic manipulation. Our calculations show that entanglement can be certified in antiferromagnetically coupled spin chains using state of the art spectral resolution of ESR-STM magnetometry.

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