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Regensburg 2025 – wissenschaftliches Programm

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HL: Fachverband Halbleiterphysik

HL 2: 2D Semiconductors and van der Waals Heterostructures I

HL 2.4: Vortrag

Montag, 17. März 2025, 10:15–10:30, H15

Current-induced second-harmonic generation in monolayer graphene-devices — •Nele Tornow1, Friederike Renz-Wieland1, Omid Ghaebi1, and Giancarlo Soavi1,21Institute of Solid State Physics, Friedrich Schiller University Jena, Jena, Germany — 2Abbe Center of Photonics, Friedrich Schiller University Jena, Jena, Germany

In pristine and isolated graphene, second-order nonlinear optical processes are, within the dipole approximation, forbidden due to the invariance under space inversion symmetry. Few studies have suggested that inversion symmetry can be broken by in-plane currents, leading to a measurable second-harmonic generation (SHG) [1,2]. In particular, investigations have shown that interfacial charge trapping between a monolayer graphene and silicon dioxide (SiO2) on silicon substrate results in electrically tunable SHG when driving in-plane currents [2]. To further verify this hypothesis, we study current-tunable second-harmonic emission in two graphene based devices: one high-quality double-encapsulated hexagonal boron nitride/graphene field-effect transistor and one with a graphene-SiO2 interface, finding SHG only in the latter one.

Our findings provide insights into the origin of current-tunable SHG and the mechanisms underlying space inversion symmetry breaking in graphene.

[1] Dean, J. et al., Appl. Phys. Lett. 26, 261910 (2009)

[2] An, Y. et al., Nano Lett. 13, 2104-2109 (2013)

Keywords: Graphene; Symmetry; Harmonic Generation

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