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MA: Fachverband Magnetismus

MA 23: Focus Session: Magneto-Transport and Magneto-Optics of Higher Orders in Magnetization I

MA 23.8: Talk

Wednesday, March 19, 2025, 12:15–12:30, H20

Anisotropy of the contributions to the orbital magnetization — •Milan Vrána1,2 and Jaroslav Hamrle1,21Charles University, Prague, Czech Republic — 2Czech Technical University, Prague, Czech Republic

The general definition of orbital magnetization is the change in the grand canonical potential, Ω, with respect to the external magnetic field: morb = −∂ Ω / ∂ B. The orbital magnetization consists of two distinct contributions [1]. The first term originates from the orbital motion of electrons and is given by mdip = −e/2 ⟨ ψ | r × v | ψ ⟩. The second term, mkden, has been reinterpreted as arising from changes in the density of k-points in phase space due to the concurrent presence of both the magnetic field and the Berry curvature, Ω [2]. This violates Liouville’s theorem, leading to an expansion or contraction of the phase space volume by a factor of (1 + e/ℏ B · Ω). In the model material bcc Fe, we demonstrate that mkden is negligible in the [100] magnetization direction, whereas mdip is negligible in the [111] direction. It demonstrates different nature of the orbital magnetization for different magnetization directions. However, the magnitude of the total orbital magnetization, morb = mdip + mkden, remains nearly independent of the magnetization direction.

Keywords: orbital magnetization; Berry curvature

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