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MM: Fachverband Metall- und Materialphysik

MM 6: Phase Transformations

MM 6.3: Talk

Monday, March 17, 2025, 16:15–16:30, H10

Magnetic-field induced phase transition crossover in the triangular-lattice antiferromagnet: Ba3CoSbO9 — •Sanjay Kumar1, Koushik Chakraborty2, Aditi Agrawal2, Shalini Mishra3, M. P. Saravanan2, Arvind Kumar Yogi2, Satyapal S. Rathore4, and Rashi Nathawat11Functional Ceramics and Smart Materials Lab, Department of Physics, Manipal University Jaipur, Jaipur - 303007, India — 2UGC-DAE Consortium for Scientific Research, University Campus, Khandwa Road, Indore-452001, India — 3Department of Physics, Govt. Holkar Science College, Indore (M.P.) 452001, India — 4Department of Physics, Cluster University of Jammu, Jammu * 180001, India

We report magnetic and structural properties of triangular-lattice antiferromagnet Ba3CoSbO9 by means of x-ray diffraction (XRD), magnetic susceptibility, specific heat, x-ray photoelectron spectroscopy (XPS), and dielectric measurements. Thermodynamic measurements show a long-range ordered (LRO) state at Néel temperature TN = 3 K which was found to be shift at higher temperatures at about TN = 4.1 K under the higher magnetic fields. Moreover, we have found higher Curie-Weiss temperature θCW ∼-133.2 K from the inverse susceptibility fit which reveals frustration parameter about  44, suggesting magnetic lattice is highly frustrated. Further, a spin-glass state signature was evident at around 6.5 K, which was found to be fully suppressed at a higher magnetic field ( H ∼16 T). Interestingly, Ba3CoSbO9 exhibits a broad maximum at around Tmax ∼5 K which becomes pronounced as the magnetic field is increased.

Keywords: Quantum Materials; X-ray diffraction; Magnetism; Frustrated lattice

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