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O: Fachverband Oberflächenphysik
O 72: Poster Plasmonics and Nanooptics: Light-Matter Interaction, Spectroscopy
O 72.9: Poster
Mittwoch, 19. März 2025, 18:00–20:00, P2
Energy and momentum distribution of surface plasmon-induced hot carriers — •Ellen Brennfleck1, Christopher Weiß1, Jannis Leßmeister1, Tobias Eul2, Benjamin Stadtmüller3, and Martin Aeschlimann1 — 1Department of Physics and Research Center OPTIMAS, University of Kaiserslautern-Landau, Germany — 2Institute of Experimental and Applied Physics, University of Kiel, Germany — 3Institute of Physics, University of Augsburg, Germany
Are the spectroscopic properties of plasmon- and photon-induced carriers fundamentally different? This question is crucial for advancing plasmonic energy conversion. Initial studies have suggested characteristic energy and momentum distributions for the photoemission of both bulk plasmon resonances and surface plasmons. For surface plasmons, however, the separation of plasmon and photon-induced emission patterns by their inherent spatial and dynamics remains challenging [1].
To further characterize the electron emission pattern of surface plasmons, we combine a femtosecond laser system with a spatial light modulator to generate a vector vortex beam to excite surface plasmon polaritons at an annular structure. Our photoemission electron microscope enables us to compare the spectroscopic properties of photoemitted electrons and those generated by plasmonic emission at the center of the structure, providing valuable insights into the distinct emission mechanisms.
[1] Hartelt et al., ACS Nano 15, 12 (2021), 19559--19569
Keywords: plasmon-induced hot carriers; surface plasmon polariton; PEEM; momentum microscopy; spatial light modulator